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Optical frequency combs have enabled distinct advantages in broadband, high-resolution spectroscopy and precision interferometry. However, quantum mechanics ultimately limits the metrological precision achievable with laser frequency combs. Quantum squeezing has led to substantial measurement improvements with continuous wave lasers, but experiments demonstrating metrological advantage with squeezed combs are less developed. Using the Kerr effect in nonlinear optical fiber, a 1-gigahertz frequency comb centered at 1560 nanometers is amplitude-squeezed by >3 decibels (dB) over a 2.5-terahertz bandwidth. Dual-comb interferometry yields mode-resolved spectroscopy of hydrogen sulfide gas with a signal-to-noise ratio nearly 3 dB beyond the shot-noise limit. The quantum noise reduction leads to a twofold quantum speedup in the determination of gas concentration, with implications for high-speed measurements of multiple species in dynamic chemical environments. 

Mid-infrared microscopy is an important tool for biological analyses, allowing a direct probe of molecular bonds in their low energy landscape. In addition to the label-free extraction of spectroscopic information, the application of broadband sources can provide a third dimension of chemical specificity. However, to enable widespread deployment, mid-infrared microscopy platforms need to be compact and robust while offering high speed, broad bandwidth, and high signal-to-noise ratio. In this study, we experimentally showcase the integration of a broadband, high-repetition-rate dual-comb spectrometer (DCS) in the mid-infrared range with a scanning microscope. We employ a set of 1-GHz mid-infrared frequency combs, demonstrating their capability for high-speed and broadband hyperspectral imaging of polymers and ovarian tissue. The system covers 1000 cm−1 at νc = 2941 cm−1 with 12.86 kHz spectra acquisition rate and 5 µm spatial resolution. Taken together, our experiments and analysis elucidate the trade-off between bandwidth and speed in DCS as it relates to microscopy. This provides a roadmap for the future advancement and application of high-repetition-rate DCS hyperspectral imaging. 

Dual-comb spectroscopy in the ultraviolet (UV) and visible would enable broad bandwidth electronic spectroscopy with unprecedented frequency resolution. However, there are significant challenges in generation, detection, and processing of dual-comb data that have restricted its progress in this spectral region. In this work, we leverage robust 1550 nm few-cycle pulses to generate frequency combs in the UV–visible. We combine these combs with a wavelength multiplexed dual-comb spectrometer and simultaneously retrieve 100 MHz comb-mode-resolved spectra over three distinct harmonics at 386, 500, and 760 nm. The experiments highlight the path to continuous dual-comb coverage spanning 200–750 nm, offering extensive access to electronic transitions in atoms, molecules, and solids. 

We demonstrate a 10 GHz octave-spanning frequency comb from a 1550 nm resonant waveguide-type electro-optic comb generator. The impact of cavity filtering on the amplified spontaneous emission and shot noise is studied experimentally and theoretically. 

We report high-speed measurements of chemical kinetics reactions inside a shock tube using a 1-GHz repetition rate mid-infrared dual-comb spectrometer. We show formation of formaldehyde and sub-sequent decomposition to carbon-monoxide with 17.5 μs time resolution. 

We demonstrate efficient 10 GHz frequency comb generation using chirped periodically poled nanophotonic lithium niobate waveguides. Spectral coverage across the UV and visible is achieved with pulse energies less than 50 pJ. 

We demonstrate thin-film lithium niobate waveguides with chirped poling periods for efficient supercontinuum viaχ⁽²⁾andχ⁽³⁾nonlinearities. With picojoule energies, we generate gap free frequency combs spanning 330 to 2400 nm. 

We employ an efficient 1550 nm resonant waveguide-type electro-optic comb generator with PM nonlinear fiber optics to generate 50 fs pulses and 500 nm broad super- continuum at 20 GHz.